Methods for determining several important parameters of partially homogeneously broadened gas lasers, such as the Lorentzian line width, Doppler line width, spontaneous emission line width, saturation intensity, and gain coefficients, have been developed for both continuous wave and pulsed operation. For CW gas lasers, values for the gain and line-shape parameters are obtained from an analysis of experimental measurements of the saturated gain at the line center vs input intensity, and of the spontaneous emission line width, based on a quadratic approximation to the saturated gain and a Voigt function description of Fabry–Perot interferograms. Line-shape parameters of a laser amplifier can also be determined by analyzing measurements of the pulse intensity gain, pulse duration time and pulse delay time, using numerically calculated functions of the ratio of Lorentzian to Doppler line width. Experimental measurements for both CW and pulsed operation of the xenon 3.5 µm laser transition are adduced and analyzed as an example.